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In situ Raman analyses of electrode materials for Li-ion batteries

Sorbonne Université, Campus Pierre et Marie Curie, Institut de Minéralogie, Physique des Matériaux et de Cosmochimie (IMPMC), UMR 7590, 4 place Jussieu, 75005 Paris, France

Topical Section: Materials Characterization

The purpose of this review is to acknowledge the current state-of-the-art and the progress of in situ Raman spectro-electrochemistry, which has been made on all the elements in lithium-ion batteries: positive (cathode) and negative (anode) electrode materials. This technique allows the studies of structural change at the short-range scale, the electrode degradation and the formation of solid electrolyte interphase (SEI) layer. We also discuss the results in the perspective of spatial and real-time investigations by in situ Raman imaging (mapping) during charge/discharge cycling.
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