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In situ Raman analyses of electrode materials for Li-ion batteries

Christian M. Julien Alain Mauger

*Corresponding author: Christian M. Julien christian.julien@upmc.fr


The purpose of this review is to acknowledge the current state-of-the-art and the progress of in situ Raman spectro-electrochemistry, which has been made on all the elements in lithium-ion batteries: positive (cathode) and negative (anode) electrode materials. This technique allows the studies of structural change at the short-range scale, the electrode degradation and the formation of solid electrolyte interphase (SEI) layer. We also discuss the results in the perspective of spatial and real-time investigations by in situ Raman imaging (mapping) during charge/discharge cycling.

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